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#2 Re: Quantum Chemistry » Second Order Perturbation Theory Analysis using Gaussian Software » 2023-06-15 10:42:22

Then how am I supposed to make comparison with other system since the other system also has a stabilization energy of 18.87 and 0.80 respectively for the same donor-acceptor pairs.
Added to this there are contributions involving s-orbital.
Here am giving an example of how the systems differ in their stabilization energy values.
System 1
donor-->p-orbital = 11.23
donor-->p-orbital = 9.06
donor-->s-orbital= 4.83

System2

donor-->p-orbital = 18.87
donor-->p-orbital = 0.80
donor-->s-orbital= 15.06

The donor orbital is the same in each case. It is a C-H sigma bond.

#3 Quantum Chemistry » Second Order Perturbation Theory Analysis using Gaussian Software » 2023-06-14 15:32:04

Anjali Ganai
Replies: 4

Hello,

I have carried out the second order perturbation analysis and a small section of the output is (showing the involved NBOs and Stabilization Energies):

21. BD(1) C 25-H 28       /121. LP*(7)Fe 30    9.06
21. BD(1) C 25-H 28       /122. LP*(8)Fe 30    11.23

Now NBO No. 121 and 122 are almost pure P orbitals as can be seen from below
121. (0.09383) LP*(7)Fe 30     s(1.96%)p49.61(97.4%)d 0.30(0.60%)f 0.00(0.00%)
122. (0.08905) LP*(8)Fe 30     s(1.16%)p84.81(98.31%)d 0.46(0.53%)f 0.00(0.00%)

My question is which of the two NBO(121 or 122 or both) should I consider? Do I need to add both values of stabilization energies (11.23+9.06) to make comparison with other systems?

Regards,
Anjali

#4 Quantum Chemistry » IRC calculation in gaussian 16 ends abnormally! » 2023-04-01 05:02:26

Anjali Ganai
Replies: 1

Hello,

I'm trying to perform an IRC calculation in Gaussian 16. IRC in the forward direction ran successfully but the calculation ended abnormally for the backward direction.

My route section reads:
#p irc=(calcfc,recorrect=never,maxpoints=12,recalc=4) um06l/gen geom=connectivity scf=xqc Integral(Grid=UltraFineGrid) NoSymmetry

The last few line of the output file is as follows:

No NMR shielding tensors so no spin-rotation constants.
Leave Link  601 at Fri Mar 31 10:02:04 2023, MaxMem=   536870912 cpu:              17.9 elap:               1.0
(Enter /apps/scratch/compile/g16/l9999.exe)

This type of calculation cannot be archived.


TWO ROADS DIVERGED IN A WOOD, AND I--
I TOOK THE ONE LESS TRAVELED BY,
AND THAT HAS MADE ALL THE DIFFERENCE.

                       -- ROBERT FROST
Job cpu time:       4 days 12 hours 53 minutes 52.7 seconds.
Elapsed time:       0 days  5 hours 27 minutes 28.6 seconds.
File lengths (MBytes):  RWF=   1311 Int=      0 D2E=      0 Chk=     24 Scr=      2
Normal termination of Gaussian 16 at Fri Mar 31 10:02:06 2023.

I cannot figure out what went wrong. Can someone please suggest what caused the error and how to get rid of it!

Regards,
Anjali

#6 Multiwfn and wavefunction analysis » Analysis of valence electron density for open-shell molecules » 2023-03-03 07:26:32

Anjali Ganai
Replies: 2

Hello,

In section 4.6.2 valence electron density analysis for closed-shell  molecules have been discussed with example.
I was wondering how the analysis of valence electron density of open-shell molecules could be carried out. It would be helpful if an example for working with open-shell moelcules could be provided.

Regards,
Anjali

#8 Re: Multiwfn and wavefunction analysis » PDOS calculation » 2023-02-22 11:28:07

Hello Sir,

I have been following part 4 of Section 4.10.1 of the manual where it is written that "Please use main function 0 of Multiwfn to visualize
corresponding MO isosurfaces." The plot for TDOS/PDOS/OPDOS shows only energies of the MOs (represented by lines at the base of the plot). Could you please say how to understand which MO/MO index should I visualize or which line corresponds to which MO index?

Regards,
Anjali

#10 Re: Quantum Chemistry » BSSE corrected binding Gibbs free energies » 2022-08-17 10:18:00

Can I use out =wfn with job type energy and pop=(full,nbo) in gaussian to generate the .wfn file for NCI analysis?

#12 Re: Quantum Chemistry » BSSE corrected binding Gibbs free energies » 2022-08-17 09:27:13

My another question is
While running the job with type 'energy' and counterpoise=2, can I add out=wfn to get the .wfn file which will be used for Non-covalent interaction (NCI) analysis  in Multiwfn? Or do I have to run two separate jobs- one for counterpoise=2 and another for wfn file which will be used for Non-covalent interaction (NCI) analysis ?

#13 Re: Quantum Chemistry » BSSE corrected binding Gibbs free energies » 2022-08-17 09:22:45

I had a question regarding BSSE corrected binding energy.
I want to calculate BSSE corrected binding energy of say A+B----> AB
I have the energies of molecules A, B and complex AB.
So, del E' = E(AB) - E(A)- E(B).
I then run a job in gaussian with type 'energy' and counterpoise=2. The .log file contains  'BSSE energy =       0.015554255487'
Will the BSSE corrected binding energy be delE'+  0.015554255487 ?

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